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- W4294295616 abstract "The odyssey of photochemistry is accompanied by the journey to manipulate electrons and protons in time, in space, and in energy. Over the past decades, single-electron (1e-) photochemical transformations have brought marvelous achievements. However, as each photon absorption typically generates only one exciton pair, it is exponentially challenging to accomplish multielectron and proton photochemical transformations. The multistep differences in thermodynamics and kinetics urgently require us to optimize light harvesting, expedite consecutive electron transfer, manipulate the interaction of catalysts with substrates, and coordinate proton transfer kinetics to furnish selective bond formations. Tandem catalysis enables orchestrating different photochemical events and catalytic transformations from subpicoseconds to seconds, which facilitates multielectron redox chemistries and brings consecutive, value-added reactivities. Joint efforts in molecular and material design, mechanistic understanding, and theoretical modeling will bring multielectron and proton synthetic opportunities for fuels, fertilizers, and chemicals with enhanced versatility, efficiency, selectivity, and scalability, thus taking better advantage of photons (i.e., sunlight) for our sustainable society." @default.
- W4294295616 created "2022-09-02" @default.
- W4294295616 creator A5001548891 @default.
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- W4294295616 creator A5031380067 @default.
- W4294295616 creator A5049301997 @default.
- W4294295616 creator A5071014155 @default.
- W4294295616 date "2022-09-02" @default.
- W4294295616 modified "2023-10-16" @default.
- W4294295616 title "Photochemistry Journey to Multielectron and Multiproton Chemical Transformation" @default.
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