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- W4294827422 abstract "The chemo- and site-selective reaction at the particular C–N amide bond among a sea of other amides is a significant and long-standing challenge. Although the use of twisted amides has been demonstrated for modifications of inert C–N amide bonds, none of these methods can selectively activate a particular amide bond for C–C bond formation in the presence of similar amides. Using density functional theory as a guide, we report the first site-selective C–C bond modification of a particular C–N amide bond in polyamides with a low twist angle by combining ground-state steric distortion with electronic activation." @default.
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- W4294827422 date "2022-09-06" @default.
- W4294827422 modified "2023-09-25" @default.
- W4294827422 title "Selective Conversion of Unactivated C–N Amide Bond to C–C bond via Steric and Electronic Resonance Destabilization" @default.
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- W4294827422 doi "https://doi.org/10.1021/acs.orglett.2c02420" @default.
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