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• W4294845148 endingPage "110694" @default.
• W4294845148 startingPage "110694" @default.
• W4294845148 abstract "Conjugated organoboranes with thermally activated delayed fluorescence (TADF) have emerged as a promising kind of organic emitting materials. In this study, we report the design of organoborane TADF emitters using double B←N bridged bipyridine (BNBP) as an electron-accepting unit. A series of novel BNBP-containing D‒A‒D-type organoboranes were facilely synthesized via the Buchwald–Hartwig amination and then borylation reactions. Their single-crystal and electronic structures, as well as photophysical and electrochemical properties were fully investigated. Notably, by varying the electron donor groups from diphenylamine and carbazole to 9,9-dimethyl-9,10-dihydroacridine, the slight overlapping between highest occupied molecular orbital and lowest unoccupied molecular orbital and small singlet-triplet energy gaps of organoborane molecule were obtained, thus leading to the intriguing TADF property. Moreover, the aggregation-induced emission characteristic was unexpected demonstrated for this organoborane molecule. A series of organoborane emitters with double B←N bridged bipyridine as the electron acceptor were synthesized, and one of them possesses thermally activated delayed fluorescence and aggregation-induced emission properties. • A series of organoborane emitters with double B←N bridged bipyridine as the electron acceptor were synthesized. • Their single-crystal structures, and electronic structures and properties were fully investigated. • One organoborane emitter possesses thermally activated delayed fluorescence and aggregation-induced emission properties." @default.
• W4294845148 created "2022-09-07" @default.
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• W4294845148 date "2022-11-01" @default.
• W4294845148 modified "2023-09-30" @default.
• W4294845148 title "Organoborane emitter containing double B←N bridged bipyridine that displays delayed fluorescence and aggregation-induced emission" @default.
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• W4294845148 doi "https://doi.org/10.1016/j.dyepig.2022.110694" @default.
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