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- W4295096262 abstract "Although low-dimensional hybrid metal halides have emerged as promising light emitters due to their broadband emission originated from self-trapped exciton (STE), the synthesis of lead-free halides with high photoluminescence quantum yield remains a challenge. Herein, a series of new luminescent single crystals of antimony-based metal halides [Na(DMSO)2]3SbBr6−xClx (x = 0, 2, 3, 4, 6) is synthesized. By optimizing the ratio of Br and Cl, [Na(DMSO)2]3SbBr3Cl3 exhibits an ultra-broadband yellow light emission peaking at 606 nm with a full width at half-maximum of 160 nm and a high photoluminescence quantum yield of 90.6%. Both experimental characterizations and theoretical calculations indicate that STE emission is responsible for the ultra-broadband yellow light emission. Furthermore, blue LED chip-pumped white light-emitting diodes by using the yellow-emitting [Na(DMSO)2]3SbBr3Cl3 are demonstrated, showing a correlated color temperature of 3948 K and a color rendering index of 85. Finally, a large-size and flexible [Na(DMSO)2]3SbBr3Cl3 scintillator used for X-ray imaging is prepared by a template assembled method, exhibiting a high spatial resolution of 15.5 lp mm−1 and a low detection limit of 285.8 nGyair s−1. This work highlights the potential of Sb-based halides in solid-state illumination and X-ray imaging." @default.
- W4295096262 created "2022-09-10" @default.
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- W4295096262 date "2022-09-08" @default.
- W4295096262 modified "2023-10-03" @default.
- W4295096262 title "High Quantum Efficiency of Stable Sb‐Based Perovskite‐Like Halides toward White Light Emission and Flexible X‐Ray Imaging" @default.
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- W4295096262 doi "https://doi.org/10.1002/adom.202201509" @default.
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