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- W4295366579 abstract "The wide use of Li-ion batteries in energy storage has resulted in a new waste product stream rich in valuable metals Mn, Ni, and Co with well-known catalytic activities. In this work, a spent Li-ion battery electrode material with lithium nickel manganese cobalt oxide is shown as an excellent reusable catalyst for oxidation of biomass-derived furan aldehydes and alcohols to their value-added oxidation products with applications in the sustainable polymer industry. A mechanically separated, combined cathode and anode black material from a spent DELL 1525 laptop battery was pyrolyzed in air at 600 °C to remove binders and electrolytes to prepare the catalyst. The SEM, XRF, and X-ray crystallography analysis of the catalyst showed the presence of C, O, Li, Ni, Co, and Mn, indicating the presence of a lithium nickel manganese cobalt oxide (LiNixMnyCozO2)-type cathode material in the spent Li-ion battery employed in the study. This material was shown as an efficient catalyst for the oxidation of aldehyde and alcohol functional groups in biofurans, furan-2-aldehyde, 5-hydroxymethyl furfural, and 5,5′-[oxybis(methylene)]bis[2-furaldehyde], to their corresponding carboxylic acids in 82–97% yield, at 120–140 °C, under 1.24 MPa oxygen, and in 0.10 M aq. Na2CO3 medium." @default.
- W4295366579 created "2022-09-13" @default.
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- W4295366579 date "2022-09-13" @default.
- W4295366579 modified "2023-10-16" @default.
- W4295366579 title "Spent Li-Ion Battery Electrode Material with Lithium Nickel Manganese Cobalt Oxide as a Reusable Catalyst for Oxidation of Biofurans" @default.
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- W4295366579 doi "https://doi.org/10.1021/acssuschemeng.2c03346" @default.
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