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• W4295681543 endingPage "111551" @default.
• W4295681543 startingPage "111551" @default.
• W4295681543 abstract "Bacterial biofilms formed on various surfaces can cause serious contamination issues, resulting in economic losses and also threatening public health. However, as a widely used protective material, polymeric gels are usually developed with effective antibacterial properties in killing planktonic bacteria rather than eradicating mature biofilms. Herein, two types of cationic sulfonium-based gels (TEE-S+ and ETT-S+) with inherent antibacterial properties were presented, which can be facilely prepared through the thiol-epoxy “click” reaction and methylation by varying the type and the proportion of precursors. All these gels displayed excellent bactericidal properties (>9-log reduction) against both planktonic Gram-negative (E. coli) and Gram-positive (S. aureus) bacteria. The series of TEE-S+ gels presented excellent efficiency in eradicating 3-day mature biofilms of E. coli (∼85 % biomass reduction) by killing embedded cells (>7-log killing efficiency), while ETT-S+ gels with the optimal composition showed outstanding eradication (75%–90% biomass reduction) and killing efficiency (>7-log) against both E. coli and S. aureus biofilm. Moreover, by tuning the crosslinking density of the gel matrix, their compressive modulus and swelling ratio can be adjusted from 5 to 120 kPa and from 17% to 800%, respectively. This work suggests sulfonium-based gels can serve as a promising candidate to provide antibacterial and antibiofilm protection in different application scenarios." @default.
• W4295681543 created "2022-09-14" @default.
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• W4295681543 date "2022-10-01" @default.
• W4295681543 modified "2023-10-11" @default.
• W4295681543 title "Development of cationic sulfonium-based gels with inherent antibacterial, excellent antibiofilm, and tunable swelling properties" @default.
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• W4295681543 doi "https://doi.org/10.1016/j.eurpolymj.2022.111551" @default.
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