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• W4295706120 abstract "Single-ion conductors have garnered attention in energy storage systems as a promising alternative to currently widespread electrolytes that allow migration of cations and anions. However, ion transport phenomena of most single-ion conductors are affected by strong ion (e.g., Li+)-ion (immobilized anionic domains) interactions and tortuous paths, which pose an obstacle to achieving performance breakthroughs. Here, we present a Li+-centered G-quadruplex (LiGQ) as a class of single-ion conductor based on directional Li+ slippage at the microscopic level. A guanine derivative with liquid crystalline moieties is self-assembled to form a hexagonal ordered columnar structure in the LiGQ, thereby yielding one-dimensional central channels that provide weak ion-dipole interaction and straightforward ionic pathways. The LiGQ exhibits weak Li+ binding energy and low activation energy for ion conduction, verifying its viability as a new electrolyte design." @default.
• W4295706120 created "2022-09-14" @default.
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• W4295706120 date "2022-09-16" @default.
• W4295706120 modified "2023-10-16" @default.
• W4295706120 title "Ion slippage through Li ⁺ -centered G-quadruplex" @default.
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• W4295706120 doi "https://doi.org/10.1126/sciadv.abp8751" @default.
• W4295706120 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36103528" @default.
• W4295706120 hasPublicationYear "2022" @default.
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