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- W4295780149 abstract "Nitrogen cycling (N 2 -NO x -NH 3 ) is essential for maintaining life as it is crucial in fertilizers and nucleic acids. However, the current NH 3 synthesis (N 2 -to-NH 3 ) for fertilizers and energy requires large amounts of fossil fuels and greenhouse gas emissions, compromising its eco-economic significance. Meanwhile, approaches like selective catalytic reaction are applied to neutralize the toxic NO x into N 2 but call for value-added NH 3 as the reduction agent. In this regard, directly converting harmful NO x , one of the major environmental pollutants, into NH 3 is a promising way to balance the nitrogen cycle eco-friendly, which is still in its infancy. Recently, the electrocatalytic NO x reduction reaction (NO x RR) unveiled a potential route for the NO x -to-NH 3 conversion. This review presents the latest progress in the electrocatalytic NO x RR in reaction mechanism and catalysts design. It will provide a comprehensive understanding to guide future research in NO x RR, aiming to offer sustainable chemistry and energy feedstocks for the carbon-zero economy. • This work overviews the electrocatalytic NO x reduction. • The possible reaction mechanism is highlighted. • Innovative concepts for catalysts design are described." @default.
- W4295780149 created "2022-09-15" @default.
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- W4295780149 date "2022-12-01" @default.
- W4295780149 modified "2023-10-18" @default.
- W4295780149 title "Enclosing the nitrogen cycle: Ammonia synthesis by NOx reduction" @default.
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- W4295780149 doi "https://doi.org/10.1016/j.cogsc.2022.100681" @default.
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