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- W4295909377 endingPage "6972" @default.
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- W4295909377 abstract "We report a general and scalable method for the synthesis of all-meta-trisubstituted benzenes from readily available 3,5-disubstituted catechols. Oxidation and [4 + 2] cycloaddition with acetylene dienophiles generate a bicyclo[2.2.2]octane structure that is doubly decarbonylated initiated by blue-light irradiation, leading to a meta,meta-disubstitution pattern on the re-aromatized system. This enables this substitution pattern even with very bulky alkyl groups (deemed excellent dispersion energy donors) to be incorporated into, for example, chiral phosphoric acid catalysts." @default.
- W4295909377 created "2022-09-16" @default.
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- W4295909377 date "2022-09-15" @default.
- W4295909377 modified "2023-10-18" @default.
- W4295909377 title "All That <i>metas</i>─Synthesis of Dispersion Energy Donor-Substituted Benzenes" @default.
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- W4295909377 doi "https://doi.org/10.1021/acs.orglett.2c02780" @default.
- W4295909377 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36107734" @default.
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