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- W4295936617 abstract "The dehydropolymerisation of phenylsilane is investigated using group 4 metallocene amide complexes as catalysts. The dinuclear zirconocene amide complex Cp2Zr(NMe2)(μ-Me3SiC3SiMe3)Zr(NMe2)Cp2 (2) (Cp = η5-cyclopentadienyl) shows high activity in dehydrocoupling reactions, producing polyphenylsilanes with molecular weights ranging from 200 to 3000 g mol-1 and linear-to-cyclic product ratios of up to 80 : 20. Likewise, different ratios of oligomers and polymers with different tacticities could be described. Ansa-zirconocene amide complexes possessing the ebthi (ebthi = 1,2-ethylene-1,1'-bis(η5-tetrahydroindenyl)) ligand systems were prepared and evaluated for catalytic dehydropolymerisation in comparison to the dinuclear catalyst system." @default.
- W4295936617 created "2022-09-16" @default.
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- W4295936617 date "2022-01-01" @default.
- W4295936617 modified "2023-09-26" @default.
- W4295936617 title "Mono- and dinuclear zirconocene(<scp>iv</scp>) amide complexes for the catalytic dehydropolymerisation of phenylsilane" @default.
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- W4295936617 doi "https://doi.org/10.1039/d2ra04955d" @default.
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