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• W4296071390 abstract "In this review, we focus on traditional carbon sources (graphite, etc.), and novel carbon sources (MXene, graphene, etc.). The merits and demerits of interfacial bonding of Si/C composites are summarized. • Various carbon sources in Si/C composites, such as traditional carbon sources like graphite, pitch, and biomass, and novel carbon sources like MXene, graphene, MOFs-derived carbon, and graphdiyne et al are reviewed and discussed. • Influence of interfacial bonding of silicon and carbon in the Si/C anodes on electrochemical performance and introduction method are explored and summarized. • Electrochemical process and morphological evolution of lithiation/delithiation of Si anodes are summarized. • Composition and micromorphology of SEI on Si anodes are summarized. • Selection of carbonaceous materials, structural design and interface control of Si/C anodes, and application of Si/C anodes in all-solid-state lithium-ion batteries and sodium-ion batteries et al. are summarizes and prospected. Silicon (Si) has been studied as a promising alloying type anode for lithium-ion batteries due to its high specific capacity, low operating potential and abundant resources. Nevertheless, huge volume expansion during alloying/dealloying processes and low electronic conductivity of Si anodes restrict their electrochemical performance. Thus, carbon (C) materials with special physical and chemical properties are applied in Si anodes to effectively solve these problems. This review focuses on current status in the exploration of Si/C anodes, including the lithiation mechanism and solid electrolyte interface formation, various carbon sources in Si/C anodes, such as traditional carbon sources (graphite, pitch, biomass), and novel carbon sources (MXene, graphene, MOFs-derived carbon, graphdiyne, etc.), as well as interfacial bonding modes of Si and C in the Si/C anodes. Finally, we summarize and prospect the selection of carbonaceous materials, structural design and interface control of Si/C anodes, and application of Si/C anodes in all-solid-state lithium-ion batteries and sodium-ion batteries et al. This review will help researchers in the design of novel Si/C anodes for rechargeable batteries." @default.
• W4296071390 created "2022-09-17" @default.
• W4296071390 creator A5000395470 @default.
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• W4296071390 creator A5090859513 @default.
• W4296071390 date "2023-01-01" @default.
• W4296071390 modified "2023-10-09" @default.
• W4296071390 title "Interfacial design of silicon/carbon anodes for rechargeable batteries: A review" @default.
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