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- W4296149659 abstract "Typically, oxidizing agents (such as H2O2) are necessitated for vanillic alcohol (VLA) conversion; nevertheless, intensive consumption of H2O2 is required due to the stoichiometric chemistry, and metal catalysts are usually required to improve conversion of VLA by H2O2. Nevertheless, for pursuing the goal of sustainability, it would be highly desired to develop an oxidizing agent-free and metal-free process which can selectively oxidize VLA to vanillic aldehyde (VAE). The aim of this study is to propose activated carbon fiber (ACF) as a highly effective catalyst for VLA conversion to VAE without using metals and oxidizing agents. At 120 °C within 30 min, ACF could enable CVLA = 100% with SVAE = 100% without using metals/oxidants. The effect of radical scavengers and ESR analyses further reveal that the oxidation of VLA to VAE by ACF could be attributed to reactive oxygen species derived from ACF-mediated aerobic reactions." @default.
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- W4296149659 date "2022-11-01" @default.
- W4296149659 modified "2023-10-16" @default.
- W4296149659 title "Oxidant-free and metal-free highly-selective catalytic production of vanillic aldehyde through activated carbon fiber-mediated aerobic oxidation" @default.
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- W4296149659 doi "https://doi.org/10.1016/j.jclepro.2022.134141" @default.
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