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- W4296467488 abstract "To reduce the reliance on fossil fuel, H2, as a clean fuel, has attracted substantial research and development activities in recent years. The traditional water splitting approach requires an applied bias of more than 1.5 V and the use of ion-selective membranes to prevent the formation of a potentially explosive H2–O2 gas mixture, resulting in increased cost and system design complexity. Here, a solar-driven H2 production process requiring a much lower applied bias of 1.05 V is reported whereby aniline (ANI) is oxidized to polyaniline (PANI) at the anode with a yield of 96% and H2 evolution reaction occurs at the cathode with a faradaic efficiency of 98.6 ± 3.9%. The process has multiple advantages including the elimination of ion-exchange membrane as PANI is a solid product that also is of substantially higher value than O2. For demonstration, a single junction perovskite solar cell and low-cost earth abundant CoP catalyst are successfully applied for this process. This process contributes to the advancement of solar-driven low-cost H2 generation coupled with co-production of a high-value product expediting the transition to a hydrogen economy." @default.
- W4296467488 created "2022-09-21" @default.
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- W4296467488 date "2022-09-20" @default.
- W4296467488 modified "2023-10-17" @default.
- W4296467488 title "Solar‐Driven Co‐Production of Hydrogen and Value‐Add Conductive Polyaniline Polymer" @default.
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- W4296467488 doi "https://doi.org/10.1002/adfm.202204807" @default.
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