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- W4296502012 abstract "Constructing a suitable heterojunction structure while maintaining a tight interface to promote the separation of photogenerated electrons is of great significance for improving the photocatalytic activity. In this paper, a new PANI/NH2-MIL-101(Fe) II-scheme heterojunction was prepared by a hydrothermal method. PANI with a porous structure was firstly obtained by the template method, and then PANI fragments were loaded on the surface of NH2-MIL-101(Fe) crystals under hydrothermal conditions to obtain a PANI/NH2-MIL-101(Fe) photocatalyst. The photocatalytic degradation of TC under simulated sunlight can reach 90% within an hour, and the maximum hydrogen evolution rate is 7040 μmol g-1 h-1 under visible light. The enhanced catalytic performance of PANI/NH2-MIL-101(Fe) was attributed to the appropriate matching of the VB and CB of PANI and NH2-MIL-101(Fe), and secondly, the coordination bonds formed between PANI and NH2-MIL-101(Fe) provided a channel for charge separation and transfer. Finally, a possible mechanism of the photocatalytic system was proposed through a free radical capture experiment and characterization analysis. More importantly, the experiment proved that the heterojunction formed by PANI and NH2-MIL-101(Fe) can achieve the effect of complementing each other, which provides a feasible idea and method for the design of efficient heterojunction photocatalysts." @default.
- W4296502012 created "2022-09-21" @default.
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- W4296502012 date "2022-01-01" @default.
- W4296502012 modified "2023-10-16" @default.
- W4296502012 title "Enhanced photocatalytic performance over PANI/NH<sub>2</sub>-MIL-101(Fe) with tight interfacial contact" @default.
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- W4296502012 doi "https://doi.org/10.1039/d2dt01680j" @default.
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