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• W4296612779 abstract "Abstract Photoelectrochemical (PEC) water splitting is considered a promising technology to produce renewable hydrogen, a clean fuel or energy carrier to replace conventional carbon‐based fossil‐fuel sources. Nevertheless, the overall solar‐to‐hydrogen efficiency and the cost‐effectiveness of this technology are still unsatisfactory for practical implementation. This can be primarily attributed to the sluggish kinetics of the anodic oxygen evolution reaction (OER) and the relatively low economic value of cogenerated O 2 production. Over the past decades, there are extensive efforts to explore more kinetically favorable photooxidation reactions, which coupled with hydrogen evolution reaction (HER) can simultaneously improve H 2 production yield and produce higher valuable alternatives to conventional O 2 . This review aims to present recent progress on the alternative anodic choices to OER. Here, the fundamental of PEC water splitting and the critical components required for this system are first shortly summarized. Then the benefits and issues of alternative photooxidation reactions including photooxidation of water to hydrogen peroxide, chlorine, alcohol, 5‐hydroxymethylfurfural, or urea oxidation when combined with the concurrent HER, are reviewed and analyzed. This review is concluded by presenting a critical evaluation of the challenges and opportunities of these alternative HER‐coupled photooxidation reactions for solar energy production and environmental treatment." @default.
• W4296612779 created "2022-09-23" @default.
• W4296612779 creator A5004061529 @default.
• W4296612779 creator A5030510871 @default.
• W4296612779 creator A5037181984 @default.
• W4296612779 creator A5042117799 @default.
• W4296612779 creator A5046945765 @default.
• W4296612779 creator A5050471439 @default.
• W4296612779 date "2022-09-22" @default.
• W4296612779 modified "2023-10-14" @default.
• W4296612779 title "Alternatives to Water Photooxidation for Photoelectrochemical Solar Energy Conversion and Green H₂ Production" @default.
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