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- W4296645168 abstract "Photocatalytic oxidation of aromatic alcohol into aromatic aldehyde using O2 has received huge attention, while the reaction that occurred in ambient air is rarely studied but follows the green-chemistry principles. Herein, spindle-shaped MIL-53(Fe)-NH2@ZnIn2S4 photocatalysts with a Z-scheme heterostructure were facilely developed for photocatalytic oxidation of aromatic alcohol in air under visible light. The benzyl alcohol conversion can be notably enhanced to 73% over the optimal MIL-53-NH2@ZnIn2S4 sample with a benzaldehyde production rate of 1825 μmol g–1 h–1. However, in the O2 atmosphere, the benzyl alcohol conversion is only 56%, indicating that O2 is not required and has an adverse effect on the reaction. The hierarchical structure and Z-scheme heterojunction of MIL-53-NH2@ZnIn2S4 impart an efficient separation and strong redox abilities of photo-induced electrons and holes, which are responsible for the impressive photocatalytic performance. This study could motivate the ingenious design of Z-scheme heterostructures for green organic conversion based on MOFs." @default.
- W4296645168 created "2022-09-23" @default.
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- W4296645168 date "2023-03-01" @default.
- W4296645168 modified "2023-10-16" @default.
- W4296645168 title "Constructing a Z-scheme Fe-MOF-based heterostructure for visible-light-driven oxidation of aromatic alcohol in ambient air" @default.
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- W4296645168 doi "https://doi.org/10.1016/j.jmst.2022.08.009" @default.
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