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- W4296773190 abstract "Two-dimensional materials and their heterostructures have opened up new possibilities for magnetism at the nanoscale. In this study, we utilize first-principles simulations to investigate the structural, electronic, and magnetic properties of $textrm{Fe}/textrm{WSe}_2/textrm{Pt}$ systems containing pristine, defective, or doped $textrm{WSe}_2$ monolayers. The proximity effects of the ferromagnetic Fe layer are studied by considering defective and vanadium-doped $textrm{WSe}_2$ monolayers. All heterostructures are found to be ferromagnetic, and the insertion of the transition-metal dichalcogenide results in a redistribution of spin orientation and an increased density of magnetic atoms due to the magnetized $textrm{WSe}_2$. There is an increase in the overall total density of states at the Fermi level due to $textrm{WSe}_2$; however, the transition-metal dichalcogenide may lose its distinct semiconducting properties due to the stronger than van der Waals coupling. Spin-resolved electronic structure properties are linked to larger spin Seebeck coefficients found in heterostructures with $textrm{WSe}_2$ monolayers." @default.
- W4296773190 created "2022-09-23" @default.
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- W4296773190 date "2022-09-20" @default.
- W4296773190 modified "2023-10-01" @default.
- W4296773190 title "Enhanced Magnetism in Heterostructures with Transition-Metal Dichalcogenide Monolayers" @default.
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- W4296773190 doi "https://doi.org/10.1021/acs.jpclett.2c01925" @default.
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