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- W4296822969 abstract "Understanding the kinetics of electron transfer reactions involves active research in physics, chemistry, biology, and nano-tech. Here, we propose a model to apply in a broader framework by establishing a connection between thermodynamics and kinetics. From a purely thermodynamic point of view, electronic transfer Marcus' theory is revisited; consequently, calculations of thermodynamic variables such as mobility, energy, and entropy are provided. More significantly, two different regimes are explicitly established. In the anomalous region, an exergonic process associated with negative heat capacity appears. Further, in the same region, mobility, energy, and entropy decrease when the temperature increases." @default.
- W4296822969 created "2022-09-24" @default.
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- W4296822969 date "2022-09-23" @default.
- W4296822969 modified "2023-10-15" @default.
- W4296822969 title "Anomalous (Exergonic) Behavior in the Transfer of Electrons between Donors and Acceptors: Mobility, Energy, Caloric Capacity, and Entropy" @default.
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- W4296822969 doi "https://doi.org/10.1021/acsomega.2c04094" @default.
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