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• W4296826777 abstract "Abstract The practical application of lithium (Li) metal anode (LMA) is still hindered by non‐uniformity of solid electrolyte interphase (SEI), formation of “dead” Li, and continuous consumption of electrolyte although LMA has an ultrahigh theoretical specific capacity and a very low electrochemical redox potential. Herein, a facile protection strategy is reported for LMA using a double layer (DL) coating that consists of a polyethylene oxide (PEO)‐based bottom layer that is highly stable with LMA and promotes uniform ion flux, and a cross‐linked polymer‐based top layer that prevents solvation of PEO layer in electrolytes. Li deposited on DL‐coated Li (DL@Li) exhibits a smoother surface and much larger size than that deposited on bare Li. The LiF/Li 2 O enriched SEI layer generated by the salt decomposition on top of DL@Li further suppresses the side reactions between Li and electrolyte. Driven by the abovementioned advantageous features, the DL@Li||LiNi 0.6 Mn 0.2 Co 0.2 O 2 cells demonstrate capacity retention of 92.4% after 220 cycles at a current density of 2.1 mA cm –2 (C/2 rate) and stability at a high charging current density of 6.9 mA cm –2 (1.5 C rate). These results indicate that the DL protection is promising to overcome the rate limitation of LMAs and high energy‐density Li metal batteries." @default.
• W4296826777 created "2022-09-24" @default.
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• W4296826777 date "2022-09-23" @default.
• W4296826777 modified "2023-10-17" @default.
• W4296826777 title "High Current‐Density‐Charging Lithium Metal Batteries Enabled by Double‐Layer Protected Lithium Metal Anode" @default.
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• W4296826777 doi "https://doi.org/10.1002/adfm.202207172" @default.
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