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- W4296876002 abstract "ZnInGaS4 heterojunction with S vacancies was prepared via the microwave hydrothermal route to boost the solar-light photocatalytic activity for water splitting and Cr (VI) reduction. The tight interface between ZnIn2S4 and ZnGa2S4 favors the rapid separation and transfer of photo-induced electron-hole pairs, and the narrowed band gap is suitable for visible-light harvesting. In addition, S vacancies serve as the adsorption sites and photons capture, leading to the efficient solar utilization. Compared with ZnIn2S4 (0.94 mmol g-1h−1) and ZnGa2S4 (0.33 mmol g-1h−1), the optimal ZnInGaS4 with a In/Ga molar ratio of 1:1 exhibits the better H2 evolution rate (4.47 mmol g-1h−1) and the apparent quantum yield of 20.16 % at wavelength of 400 nm. The removal efficiency of ZnInGaS4 for solar-light driven Cr (VI) reduction is 99.46 % within 140 min, which is higher than ZnIn2S4 (93.14 %) and ZnGa2S4 (89.31 %). The photo-corrosion induces to the deactivation of ZnGa2S4 for solar-light driven H2 evolution and Cr (VI) reduction after five cycles." @default.
- W4296876002 created "2022-09-24" @default.
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- W4296876002 date "2023-01-01" @default.
- W4296876002 modified "2023-10-14" @default.
- W4296876002 title "ZnInGaS4 heterojunction with sulfide vacancies for efficient solar-light photocatalytic water splitting and Cr(VI) reduction" @default.
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- W4296876002 doi "https://doi.org/10.1016/j.cej.2022.139386" @default.
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