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- W4297200042 endingPage "121945" @default.
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- W4297200042 abstract "Surface single atom Ni-coordinated carbon nitride fibers (Ni/C3N4Fs) were reassembled into tiny NiP nanoparticle-integrated C3N4Fs (NiP/C3N4Fs) with the strengthened polarized electric fields accompanied by a weakened interface barrier. Photogenerated e- and h+ dynamically transfer to the convex-integrated NiP and concave of C3N4Fs under the synergetic electric fields via inner single atoms of Ni as charge transfer bridges within C3N4Fs interlayers, which is confirmed by high-angle annular dark field scanning transmission electron microscopy, K-edge extended X-ray absorption fine structure, X-ray photoelectron spectroscopy and theoretical prediction. H2- and O2-evolution rates of 1.89 and 0.92 mmol g−1 h−1 with solar-to-hydrogen efficiency of 2.33% are obtained over NiP/C3N4Fs system under visible light irradiation. This research provides a rational strategy for constructing the connection of H2 fuel production with its practical application." @default.
- W4297200042 created "2022-09-27" @default.
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- W4297200042 date "2023-01-01" @default.
- W4297200042 modified "2023-10-13" @default.
- W4297200042 title "Efficiently photocatalytic H2O overall splitting within the strengthened polarized field by reassembling surface single atoms" @default.
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- W4297200042 doi "https://doi.org/10.1016/j.apcatb.2022.121945" @default.
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