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- W4297222077 startingPage "2204487" @default.
- W4297222077 abstract "Solid-state alkaline metal batteries are highly sought out for their improved energy density and security over the current lithium-ion batteries. However, their practical application is heavily hindered by the interfacial issues originating from the solid electrolyte/electrode mismatch. This work demonstrates that a CuO coating layer as an active interphase can thoroughly promote the intimate contact between a Na3Zr2Si2PO12 solid electrolyte and a Na metal anode through an in situ conversion reaction. The resultant Cu/Na2O matrix forms a mixed electron/ion conducting scaffold, which facilitates stable and homogeneous Na metal plating without dendrite formation. Moreover, the symmetric Na metal cell realizes impressively steady plating/stripping cycles for 5000 h even under a high current density of 0.3 mA cm−2. The novelty is further manifested as a room-temperature solid-state Na metal full battery of Na3V1.5Al0.5(PO4)3|CuO@NZSPO|Na is assembled and exhibits a highly reversible cyclability (99.85% coulombic efficiency and 99.0% capacity retention) under a charge/discharge rate of 5 C for 2250 cycles. This work effectively solves the interfacial issues at the Na metal/solid electrolyte interface and provides a convenient way toward high-performance solid-state Na metal batteries operated at room temperature." @default.
- W4297222077 created "2022-09-28" @default.
- W4297222077 creator A5033070120 @default.
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- W4297222077 date "2022-09-26" @default.
- W4297222077 modified "2023-10-18" @default.
- W4297222077 title "Uniform Na Metal Plating/Stripping Design for Highly Reversible Solid‐State Na Metal Batteries at Room Temperature" @default.
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- W4297222077 doi "https://doi.org/10.1002/smll.202204487" @default.
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