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- W4297251570 abstract "We report, for the first time, highly crystalline cyanurate-linked covalent organic frameworks synthesized via dynamic nucleophilic aromatic substitution. The high crystallinity is enabled by the bond exchange reaction (self-correction) between 2,4,6-triphenoxy-1,3,5-triazine and diphenols via reversible SNAr catalyzed by triazabicyclodecene. The CN-COFs contain flexible backbones that exhibit a unique AA'-stacking due to interlayer hydrogen bonding interactions. The isoreticular expansion study demonstrates the general applicability of this synthetic method. The resulting CN-COFs exhibited good stability, as well as high CO2/N2 selectivity." @default.
- W4297251570 created "2022-09-28" @default.
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- W4297251570 date "2022-09-27" @default.
- W4297251570 modified "2023-10-17" @default.
- W4297251570 title "Cyanurate-Linked Covalent Organic Frameworks Enabled by Dynamic Nucleophilic Aromatic Substitution" @default.
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- W4297251570 doi "https://doi.org/10.1021/jacs.2c00778" @default.
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