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- W4297498753 abstract "The stereoselective synthesis of geometrical iron(II) complexes bearing azine-NHC ligands is described. Facial and meridional selectivity is achieved as a function of the steric demand of the azine unit, with no remarkable influence of the carbene nature. More specifically, meridional complexes are obtained upon selecting bulky 5-mesityl-substituted pyridyl coordinating units. Unexpectedly, increase of the steric hindrance in the α position with respect to the N coordinating atom results in an exclusive facial configuration, which is in stark contrast to the meridional selectivity induced by other reported α-substituted bidentate ligands. Investigation of the structure and the optical and electrochemical properties of the here-described complexes has revealed the non-negligible effect of the fac/mer ligand configuration around the metal center." @default.
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- W4297498753 date "2022-09-28" @default.
- W4297498753 modified "2023-10-13" @default.
- W4297498753 title "Substituent-Induced Control of <i>fac</i>/<i>mer</i> Isomerism in Azine-NHC Fe(II) Complexes" @default.
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- W4297498753 doi "https://doi.org/10.1021/acsorginorgau.2c00038" @default.
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