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• W4297516515 endingPage "3390" @default.
• W4297516515 startingPage "3390" @default.
• W4297516515 abstract "The stability and wide temperature performance range of solid electrolytes are the keys to the development of high-energy density all-solid-state lithium-ion batteries. In this work, a PVDF-HFP-LiClO4-Li6.4La3Zr1.4Ta0.6O12 (LLZTO) composite solid electrolyte was prepared using the solution pouring method. The PVDF-HFP-LiClO4-LLZTO composite solid electrolyte shows excellent electrochemical performance in the temperature range of 30 to 60 °C. By assembling this electrolyte into the battery, the LiFePO4/PVDF-HFP-LiClO4-LLZTO/Li battery shows outstanding electrochemical performance in the temperature range of 30 to 60 °C. The ionic conductivity of the composite electrolyte membrane at 30 °C and 60 °C is 5.5 × 10-5 S cm-1 and 1.0 × 10-5 S cm-1, respectively. At a current density of 0.2 C, the LiFePO4/PVDF-HFP-LiClO4-LLZTO/Li battery shows a high initial specific discharge capacity of 133.3 and 167.2 mAh g-1 at 30 °C and 60 °C, respectively. After 50 cycles, the reversible electrochemical capacity of the battery is 121.5 and 154.6 mAh g-1 at 30 °C and 60 °C; the corresponding capacity retention rates are 91.2% and 92.5%, respectively. Therefore, this work provides an effective strategy for the design and preparation of solid-state lithium-ion batteries." @default.
• W4297516515 created "2022-09-29" @default.
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• W4297516515 date "2022-09-28" @default.
• W4297516515 modified "2023-09-27" @default.
• W4297516515 title "Electrochemical Performance of a PVDF-HFP-LiClO4-Li6.4La3.0Zr1.4Ta0.6O12 Composite Solid Electrolyte at Different Temperatures" @default.
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• W4297516515 doi "https://doi.org/10.3390/nano12193390" @default.
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