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• W4297541510 endingPage "164501" @default.
• W4297541510 startingPage "164501" @default.
• W4297541510 abstract "The nonlinear dielectric effect (NDE) is traditionally viewed as originating from saturation of the response of individual dipoles in a strong electric field. This mean-field view, mathematically described by the Langevin saturation function, predicts enhanced dielectric saturation at lower temperatures. In contrast, recent experiments for glycerol have shown a sharp increase of the NDE with increasing temperature. The formalism presented here splits the NDE into a sum of a term representing binary correlations of dipolar orientations and terms referring to three- and four-particle orientational correlations. Analysis of experimental data shows that the contribution of three- and four-particle correlations strongly increases at elevated temperatures. The mean-field picture of dielectric saturation as the origin of the NDE is inconsistent with observations. A positive NDE (increment of the field-dependent dielectric constant) is predicted for low-concentration solutions of polar molecules in nonpolar solvents. The dependence of the NDE on the concentration of the polar component is polynomial." @default.
• W4297541510 created "2022-09-29" @default.
• W4297541510 creator A5003059556 @default.
• W4297541510 date "2022-10-28" @default.
• W4297541510 modified "2023-09-26" @default.
• W4297541510 title "Multiparticle orientational correlations are responsible for the nonlinear dielectric effect: Analysis of temperature-dependent measurements for glycerol" @default.
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• W4297541510 doi "https://doi.org/10.1063/5.0106766" @default.
• W4297541510 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36319416" @default.
• W4297541510 hasPublicationYear "2022" @default.
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