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- W4297887645 abstract "Developing cost-effective and facile methods to synthesize efficient and stable electrocatalysts for large-scale water splitting is highly desirable but remains a significant challenge. In this study, a facile ambient temperature synthesis of hierarchical nickel–iron (oxy)hydroxides nanosheets on iron foam (FF-FN) with both superhydrophilicity and superaerophobicity is reported. Specifically, the as-fabricated FF-FN electrode demonstrates extraordinary oxygen evolution reaction (OER) activity with an ultralow overpotential of 195 mV at 10 mA cm−2 and a small Tafel slope of 34 mV dec−1 in alkaline media. Further theoretical investigation indicates that the involved lattice oxygen in nickel–iron-based-oxyhydroxide during electrochemical self-reconstruction can significantly reduce the OER reaction overpotential via the dominated lattice oxygen mechanism. The rechargeable Zn–air battery assembled by directly using the as-prepared FF-FN as cathode displays remarkable cycling performance. It is believed that this work affords an economical approach to steer commercial Fe foam into robust electrocatalysts for sustainable energy conversion and storage systems." @default.
- W4297887645 created "2022-10-01" @default.
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- W4297887645 date "2023-02-10" @default.
- W4297887645 modified "2023-09-27" @default.
- W4297887645 title "Ambient Fast Synthesis of Superaerophobic/Superhydrophilic Electrode for Superior Electrocatalytic Water Oxidation" @default.
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- W4297887645 doi "https://doi.org/10.1002/eem2.12462" @default.
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