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- W4298113313 abstract "Designing an optimum separator configuration that can address severe lithium polysulfide (LiPS) shuttling and uncontrollable Li dendrite growth at the evaluated temperature is imperative for developing a high-performance, reliable, and safe Li–S battery (LSB). Herein, a promising LSB separator design is proposed, which consists of LiPS catalytic layer (LCL) and thermal conductive layer (TCL) fabricated by dual side filtrating the flower-like vanadium pentoxide (V2O5) microspheres and aluminum oxide (Al2O3) nanosheets, respectively. The LCL between the separator and S-cathode as combined LiPS trapper and catalyst significantly improves the redox reaction and sulfur utilization. At the anode/separator interface, the TCL uniforms Li-ion flux and thermal distribution to prevent undesirable Li dendrite growth under the temperature gradient (TG) effect. The Janus-type LCL-TCL separator with two parallel functions can achieve synchronous improvements in cathodic and anodic performance in LSB. Consequently, the LSB with Janus-type LCL-TCL separator exhibits excellent cycling stability with an ultralow capacity decay rate of 0.036% per cycle over 2000 cycles at 1C and superior rate capability up to 4C. The novel strategy can pave a new way to simultaneously tackle the limitations faced by anode and cathode in LSB." @default.
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- W4298113313 date "2022-12-01" @default.
- W4298113313 modified "2023-10-16" @default.
- W4298113313 title "All-in-one Janus separator for lithium–sulfur batteries with lithium polysulfide and dendrite growth suppressed at temperature gradient effect" @default.
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- W4298113313 doi "https://doi.org/10.1016/j.jpowsour.2022.232115" @default.
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