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• W4298140682 abstract "In mixtures of amines with carboxylic acids, the limited ionicity at 1:1 stoichiometric mixtures is due to insufficient ionization or ion pairing in low-dielectric environments. Higher conductivities have historically been seen at roughly 4:1 acid/base mixing ratios, where simulations have revealed large (and thus more stable) ions: homoassociated anions (AH)(AH)(A − )(HA)(HA) and cationic triple ions (BH + )(AH)(A − )(HA)(HB + ). Recent work in understanding the Gibbs energies for degree-of-ionization equilibria hints that there may be an onset, for systems with an acid-base pK a difference increasing towards 10, for the formation of free (unpaired) protonate-amine cations BH + . The transition with increasing ΔpK a is explored in this work, to aid in the prediction of ionicity and conductivity of protic ionic liquids." @default.
• W4298140682 created "2022-10-01" @default.
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• W4298140682 date "2022-09-30" @default.
• W4298140682 modified "2023-09-26" @default.
• W4298140682 title "The Transition (vs ΔpK_a) from Triple Ions to Free Cations in Poor Protic Ionic Liquids Made from Weak Acids" @default.
• W4298140682 doi "https://doi.org/10.1149/10914.0011ecst" @default.
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