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- W4299424716 abstract "Femtosecond time-resolved stimulated Raman spectroscopy is a promising method of observing the structural dynamics of short-lived transients with near infrared (near-IR) transitions, because it can overcome the low sensitivity of spontaneous Raman spectrometers in the near-IR region. Here, we describe technical details of a femtosecond time-resolved near-IR multiplex stimulated Raman spectrometer that we have recently developed. A description of signal generation and optimization, measurement, data acquisition, and calibration and correction of recorded data is provided as well. We present an application of our spectrometer to analyze the excited-state dynamics of β-carotene in toluene solution. A C=C stretch band of β-carotene in the second lowest excited singlet (S2) state and the lowest excited singlet (S1) state is clearly observed in the recorded time-resolved stimulated Raman spectra. The femtosecond time-resolved near-IR stimulated Raman spectrometer is applicable to the structural dynamics of π-conjugate systems from simple molecules to complex materials." @default.
- W4299424716 created "2022-10-02" @default.
- W4299424716 creator A5036589908 @default.
- W4299424716 creator A5043258984 @default.
- W4299424716 date "2020-02-10" @default.
- W4299424716 modified "2023-09-27" @default.
- W4299424716 title "Ultrafast Time-resolved Near-IR Stimulated Raman Measurements of Functional π-conjugate Systems" @default.
- W4299424716 doi "https://doi.org/10.3791/60437-v" @default.
- W4299424716 hasPublicationYear "2020" @default.
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