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- W4300687956 abstract "High energy demand results in comprehensive research of novel materials for energy sources and storage applications. Covalent organic frameworks (COFs) possess appropriate features such as long-range order, permanent porosity, tunable pore size, and ion diffusion pathways to be competitive electrode materials. Herein, we present a deep electrochemical study of two COF-aerogels shaped into flexible COF-electrodes (ECOFs) by a simple compression method to fabricate an electrochemical double-layer capacitor (EDLC). This energy storage system has considerable interest owing to its high-power density and long cycle life compared with batteries. Our result confirmed the outstanding behavior of ECOFs as EDLC devices with a capacity retention of almost 100 % after 10 000 charge/discharge cycles and, to our knowledge, the highest areal capacitance (9.55 mF cm-2 ) in aqueous electrolytes at higher scan rates (1000 mV s-1 ) for COFs. More importantly, the hierarchical porosity observed in the ECOFs increases ion transport, which permits a fast interface polarization (low τ0 values). The complete sheds light on using ECOFs as novel electrode material to fabricate EDLC devices." @default.
- W4300687956 created "2022-10-04" @default.
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- W4300687956 date "2022-10-25" @default.
- W4300687956 modified "2023-10-16" @default.
- W4300687956 title "Electrochemical Double‐Layer Capacitor based on Carbon@ Covalent Organic Framework Aerogels" @default.
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- W4300687956 doi "https://doi.org/10.1002/anie.202213106" @default.
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