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• W4304127975 abstract "Solar absorbers are the heart of sustainable photothermal utilization. To obtain higher photothermal conversion efficiency, nanomultilayer absorbers with low emissivity are undoubtedly the best choice. However, the strategy of co-sputtering with at least two targets is usually employed, which makes the preparation process complex and costly, so it is necessary to develop a one-step sputtering preparation through a target. Herein, we propose preparation of Ti–TiO x nanomultilayer solar selective absorption coatings (SSACs) with a single metal Ti target by one-step sputtering. The self-doped Ti nanoparticles as well as the Ti 2+ , Ti 3+ and Ti 4+ oxides in TiO x matrix can easily customize the band gap from ultraviolet to visible light, resulting in a high absorption of 0.92 and a low thermal emissivity of 0.07 (298.15K). The obtained Ti – TiO x SSACs exhibit excellent thermal stability after heat treatment at 250 °C for 300 h in air. More significantly, the measured surface temperature reached 114.5 °C under 1.5 suns simulated illumination, indicating its outstanding solar-thermal conversion ability. This work extends the application range of the titanium oxide, developing a simple method for designing low-emissivity solar absorbers. • Self-doped Ti–TiO x films with α of 0.92 and ε of 0.07 were constructed by one-step sputtering for selective absorption. • It shows good thermal stability after annealing at 250 °C and can reach 114.5 °C under indoor simulation of 1.5 suns. • This work provides an unprecedented method to achieve adjustment of selective absorption of broadband gap materials." @default.
• W4304127975 created "2022-10-11" @default.
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• W4304127975 date "2023-02-01" @default.
• W4304127975 modified "2023-09-27" @default.
• W4304127975 title "Self-doped Ti–TiOx nanomultilayer films as low-emissivity absorber by one-step sputtering" @default.
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• W4304127975 doi "https://doi.org/10.1016/j.ceramint.2022.10.083" @default.
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