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- W4304607677 abstract "Enantioselective imine reduction of dihydro-β-carbolines (DHBCs) is a reliable and powerful tool to construct bioactive chiral tetrahydro-β-carbolines (THBCs). Here, we report an efficient enantioselective imine reduction employing in situ generated Fe-thiosquaramides (Fe-TSQs) 3a and 3b as asymmetric organometallic catalysts to produce chiral THBCs (2a-h). The catalyst 3a at 15 mol % was found to be suitable for the substrates with alkyl and aryl groups which afford corresponding chiral THBCs with excellent enantioselectivities (up to ee 99%)." @default.
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- W4304607677 date "2022-10-11" @default.
- W4304607677 modified "2023-10-17" @default.
- W4304607677 title "Enantioselective Imine Reduction of Dihydro-β-carbolines by Fe-Thiosquaramide Catalyst" @default.
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- W4304607677 doi "https://doi.org/10.1021/acs.orglett.2c03093" @default.
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