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- W4304687581 abstract "Abstract Dipolar coupled multi‐spin systems have the potential to be used as molecular qubits. Herein we report the synthesis of a molecular multi‐qubit model system with three individually addressable, weakly interacting, spin centres of differing g ‐values. We use pulsed Electron Paramagnetic Resonance (EPR) techniques to characterise and separately address the individual electron spin qubits; Cu II , Cr 7 Ni ring and a nitroxide, to determine the strength of the inter‐qubit dipolar interaction. Orientation selective Relaxation‐Induced Dipolar Modulation Enhancement (os‐RIDME) detecting across the Cu II spectrum revealed a strongly correlated Cu II ‐Cr 7 Ni ring relationship; detecting on the nitroxide resonance measured both the nitroxide and Cu II or nitroxide and Cr 7 Ni ring correlations, with switchability of the interaction based on differing relaxation dynamics, indicating a handle for implementing EPR‐based quantum information processing (QIP) algorithms." @default.
- W4304687581 created "2022-10-12" @default.
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- W4304687581 date "2022-10-12" @default.
- W4304687581 modified "2023-10-14" @default.
- W4304687581 title "Modelling Conformational Flexibility in a Spectrally Addressable Molecular Multi‐Qubit Model System" @default.
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- W4304687581 doi "https://doi.org/10.1002/ange.202207947" @default.
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