Matches in SemOpenAlex for { <https://semopenalex.org/work/W4304687594> ?p ?o ?g. }
- W4304687594 endingPage "498" @default.
- W4304687594 startingPage "487" @default.
- W4304687594 abstract "For the treatment of antibiotics contained wastewater, developing a highly efficient catalyst is key to peroxymonosulfate (PMS) activation and antibiotics degradation. In this work, nitrogen-doped carbon nanosheets (NCS) coated sintered metal fibers (SMFs) catalyst was designed and developed, which could positively promote the contacting efficiency between PMS, TC and catalysts. In specific, by the dip-coating of SMFs in the cobalt-contained dicyandiamide formaldehyde resin and the following pyrolyzing coordinated polymer procedure, it was possible to create a Co-doped NCS catalyst supported on SMFs. NCS with abundant exposed surface active sites could result in a relatively higher catalytic activity. Microscopy studies confirmed the presence of stacked NCS with high Co active sites loading, which was anchored on the surface of SMFs. The developed Co NCS/SMFs catalyst exhibited a highly degradation efficiency of 96% in 240 min. Effects of operating parameters (including PMS concentration and solution pH) on the TC elimination efficicency were also investigated. Additionally, Co NCS/SMFs exhibited good PMS activation activity in the wide pH range of 2.0–9.0, and acceptable recyclability with over 86% TC removal efficiency after five cycles test. According to SEM, XRD and XPS results, highly exposed active metal sites, O defects, Co-Nx sites and reactivity of Co0 in Co NCS/SMFs played an important role in the enhancement of degradation efficiency. Finally, radical inhibition experiment and corresponding EPR test revealedthe presence of SO4∙−, ∙OH, O2∙− and 1O2 in the TC degradation system, in which singlet oxygen (1O2) was demonstrated to be the dominating reactive species for PMS activation and TC degradation. This work provided an efficient strategy for developing robust monolithic lamellar catalyst for the continuous PMS activated degradation of TC." @default.
- W4304687594 created "2022-10-12" @default.
- W4304687594 creator A5008599015 @default.
- W4304687594 creator A5017837558 @default.
- W4304687594 creator A5053272104 @default.
- W4304687594 creator A5068766717 @default.
- W4304687594 creator A5070350685 @default.
- W4304687594 creator A5080042635 @default.
- W4304687594 creator A5084496571 @default.
- W4304687594 date "2022-12-01" @default.
- W4304687594 modified "2023-09-29" @default.
- W4304687594 title "Co-doped carbon nitride nanosheets supported on SMFs for peroxymonosulfate activation to degrade tetracycline" @default.
- W4304687594 cites W1138025054 @default.
- W4304687594 cites W2044381960 @default.
- W4304687594 cites W2072038814 @default.
- W4304687594 cites W2323742690 @default.
- W4304687594 cites W2326213926 @default.
- W4304687594 cites W2413038642 @default.
- W4304687594 cites W2783426051 @default.
- W4304687594 cites W2792676415 @default.
- W4304687594 cites W2804345450 @default.
- W4304687594 cites W2809062781 @default.
- W4304687594 cites W2966153984 @default.
- W4304687594 cites W3005303359 @default.
- W4304687594 cites W3012507460 @default.
- W4304687594 cites W3013417911 @default.
- W4304687594 cites W3013795837 @default.
- W4304687594 cites W3027206052 @default.
- W4304687594 cites W3043171272 @default.
- W4304687594 cites W3091707032 @default.
- W4304687594 cites W3094777310 @default.
- W4304687594 cites W3094965389 @default.
- W4304687594 cites W3105639591 @default.
- W4304687594 cites W3113043164 @default.
- W4304687594 cites W3119681392 @default.
- W4304687594 cites W3121630377 @default.
- W4304687594 cites W3149542680 @default.
- W4304687594 cites W3162428500 @default.
- W4304687594 cites W3166988675 @default.
- W4304687594 cites W3169336166 @default.
- W4304687594 cites W3174075754 @default.
- W4304687594 cites W3195861258 @default.
- W4304687594 cites W3196279190 @default.
- W4304687594 cites W3196641822 @default.
- W4304687594 cites W3199335343 @default.
- W4304687594 cites W3202462003 @default.
- W4304687594 cites W3203855585 @default.
- W4304687594 cites W3204738418 @default.
- W4304687594 cites W3206126527 @default.
- W4304687594 cites W3208867584 @default.
- W4304687594 cites W3209537840 @default.
- W4304687594 cites W3210749368 @default.
- W4304687594 cites W3217349302 @default.
- W4304687594 cites W4200409810 @default.
- W4304687594 cites W4200471348 @default.
- W4304687594 cites W4200601458 @default.
- W4304687594 cites W4210973388 @default.
- W4304687594 cites W4213353856 @default.
- W4304687594 cites W4214489751 @default.
- W4304687594 cites W4220676201 @default.
- W4304687594 cites W4220973297 @default.
- W4304687594 cites W4220986830 @default.
- W4304687594 cites W4223933780 @default.
- W4304687594 cites W4226166932 @default.
- W4304687594 cites W4280546350 @default.
- W4304687594 cites W4281751036 @default.
- W4304687594 cites W4286208090 @default.
- W4304687594 doi "https://doi.org/10.1016/j.psep.2022.10.014" @default.
- W4304687594 hasPublicationYear "2022" @default.
- W4304687594 type Work @default.
- W4304687594 citedByCount "2" @default.
- W4304687594 countsByYear W43046875942023 @default.
- W4304687594 crossrefType "journal-article" @default.
- W4304687594 hasAuthorship W4304687594A5008599015 @default.
- W4304687594 hasAuthorship W4304687594A5017837558 @default.
- W4304687594 hasAuthorship W4304687594A5053272104 @default.
- W4304687594 hasAuthorship W4304687594A5068766717 @default.
- W4304687594 hasAuthorship W4304687594A5070350685 @default.
- W4304687594 hasAuthorship W4304687594A5080042635 @default.
- W4304687594 hasAuthorship W4304687594A5084496571 @default.
- W4304687594 hasConcept C127413603 @default.
- W4304687594 hasConcept C13965031 @default.
- W4304687594 hasConcept C161790260 @default.
- W4304687594 hasConcept C175708663 @default.
- W4304687594 hasConcept C178790620 @default.
- W4304687594 hasConcept C179104552 @default.
- W4304687594 hasConcept C185592680 @default.
- W4304687594 hasConcept C192562407 @default.
- W4304687594 hasConcept C2777492770 @default.
- W4304687594 hasConcept C2779679103 @default.
- W4304687594 hasConcept C41008148 @default.
- W4304687594 hasConcept C42360764 @default.
- W4304687594 hasConcept C515602321 @default.
- W4304687594 hasConcept C65165184 @default.
- W4304687594 hasConcept C76155785 @default.
- W4304687594 hasConceptScore W4304687594C127413603 @default.
- W4304687594 hasConceptScore W4304687594C13965031 @default.
- W4304687594 hasConceptScore W4304687594C161790260 @default.