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- W4304688607 abstract "We herein report a method for divergent copper salt controlled reactions of donor-acceptor cyclopropanes and N-fluorobenzene sulfonimide (NFSI). Specifically, in the presence of CuX2 (X=Cl, Br), the cyclopropanes underwent formal umpolung 1,3-aminohalogenation bifunctionalization via a free radical mediated ring-opening process to afford 1,3-aminochlorination and 1,3-aminobromination products in moderate to good yields. In addition, by using CuI as a catalyst, we synthesized various aminoindane derivatives via 1,3-aminoarylation cyclization of D-A cyclopropanes, the reactions involved a free radical mediated ring-opening and subsequent ring expansion via C-H bond activation." @default.
- W4304688607 created "2022-10-12" @default.
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- W4304688607 date "2022-11-22" @default.
- W4304688607 modified "2023-10-16" @default.
- W4304688607 title "Divergent Copper‐salt‐controlled Reactions of Donor‐Acceptor Cyclopropanes and <i>N</i>‐Fluorobenzene Sulfonimide: Access to the 1,3‐Haloamines and Aminoindanes" @default.
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- W4304688607 doi "https://doi.org/10.1002/chem.202202544" @default.
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