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- W4304893201 abstract "High-performance van der Waals (vdW) integrated electronics and spintronics require reliable current-carrying capacity. However, it is challenging to achieve high current density and air-stable performance using vdW metals owing to the fast electrical breakdown triggered by defects or oxidation. Here, we report that spin-orbit interacted synthetic PtTe2 layers exhibit significant electrical reliability and robustness in ambient air. The 4-nm-thick PtTe2 synthesized at a low temperature (∼400°C) shows intrinsic metallic transport behavior and a weak antilocalization effect attributed to the strong spin-orbit scattering. Remarkably, PtTe2 sustains a high current density approaching ≈31.5 MA cm-2, which is the highest value among electrical interconnect candidates under oxygen exposure. Electrical failure is caused by the Joule heating of PtTe2 rather than defect-induced electromigration, which was achievable by the native TeOx passivation. The high-quality growth of PtTe2 and the investigation of its transport behaviors lay out essential foundations for the development of emerging vdW spin-orbitronics." @default.
- W4304893201 created "2022-10-13" @default.
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- W4304893201 date "2022-11-01" @default.
- W4304893201 modified "2023-10-14" @default.
- W4304893201 title "Air-stable van der Waals PtTe2 conductors with high current-carrying capacity and strong spin-orbit interaction" @default.
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- W4304893201 doi "https://doi.org/10.1016/j.isci.2022.105346" @default.
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