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- W4306167250 abstract "Abstract Chemical transformation of polyaromatic hydrocarbon (PAH) molecules following different reaction strategies has always been the focus of organic synthesis. In this work, we report the synthesis of a PAH molecule, formation of which consists of an unusual C−C bond cleavage accompanied by a complex π‐conjugated molecular scaffold rearrangement. We demonstrate that the complex chemical transformation is steered by concerted motion of individual Au 0 gold atoms on a supporting Au(111) surface. This observation underpins the importance of single‐atom catalysis mediated by adatoms in on‐surface synthesis as well as catalytic activity of single Au 0 atoms facilitating cleavage of covalent carbon bonds." @default.
- W4306167250 created "2022-10-14" @default.
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- W4306167250 date "2022-11-15" @default.
- W4306167250 modified "2023-10-17" @default.
- W4306167250 title "Unusual Scaffold Rearrangement in Polyaromatic Hydrocarbons Driven by Concerted Action of Single Gold Atoms on a Gold Surface" @default.
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- W4306167250 doi "https://doi.org/10.1002/ange.202208010" @default.
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