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- W4306173799 abstract "MoS 2 /Ag-ZnFe 2 O 4 Z-scheme heterojunction with exposed crystal facets, Ag-doping and oxygen vacancies was used for highly efficient photocatalytic degradation of organic pollutants. • The {001}/{111} facet-based heterojunctions promote the photocatalytic activity. • The concentration of crystal defects directly relates to the number and type of crystal facets. • Z-scheme mechanism contributes more to the photocatalytic activity than crystal facets and defects. • The synergistic effect is deeply investigated by spectroscopic characterizations and theoretical calculation. Defect engineering, exposed crystal facets, and Z-scheme mechanism are promising strategies to greatly promote photocatalytic performance. Herein, the ZnFe 2 O 4 (ZFO) with Ag-doping, oxygen vacancies and different exposed crystal facets was firstly prepared by a facile hydrothermal strategy. Subsequently, the MoS 2 flowers were in-situ grown on the surface of the prepared Ag-doping ZFO (Ag-ZFO) for fabricating MoS 2 /Ag-ZFO Z-scheme heterojunction by hydrothermal strategy. Due to the synergistic effects of defect engineering (Ag-doping and oxygen vacancies), exposed crystal facets, and Z-scheme mechanism, the photocatalytic activity for tetracycline degradation was evidently improved. More importantly, the prepared MoS 2 /Ag-ZFO (T) also show excellent photocatalytic performance under real environment water. This work offers a new insight for future design and development of highly active photocatalysts." @default.
- W4306173799 created "2022-10-14" @default.
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- W4306173799 date "2023-02-01" @default.
- W4306173799 modified "2023-10-14" @default.
- W4306173799 title "Photocatalytic degradation of organic pollutants over MoS2/Ag-ZnFe2O4 Z-scheme heterojunction: Revealing the synergistic effects of exposed crystal facets, defect engineering, and Z-scheme mechanism" @default.
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- W4306173799 doi "https://doi.org/10.1016/j.cej.2022.139775" @default.
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