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- W4306249510 abstract "Abstract Layered double oxides (LDOs) can restore the parent layered double hydroxides (LDHs) structure under hydrous conditions, and this “memory effect” plays a critical role in the applications of LDHs, yet the detailed mechanism is still under debate. Here, we apply a strategy based on ex situ and in situ solid-state NMR spectroscopy to monitor the Mg/Al-LDO structure changes during recovery at the atomic scale. Despite the common belief that aqueous solution is required, we discover that the structure recovery can occur in a virtually solid-state process. Local structural information obtained with NMR spectroscopy shows that the recovery in aqueous solution follows dissolution-recrystallization mechanism, while the solid-state recovery is retro-topotactic, indicating a true “memory effect”. The amount of water is key in determining the interactions of water with oxides, thus the memory effect mechanism. The results also provide a more environmentally friendly and economically feasible LDHs preparation route." @default.
- W4306249510 created "2022-10-15" @default.
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- W4306249510 date "2022-10-14" @default.
- W4306249510 modified "2023-10-03" @default.
- W4306249510 title "Insights into memory effect mechanisms of layered double hydroxides with solid-state NMR spectroscopy" @default.
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- W4306249510 doi "https://doi.org/10.1038/s41467-022-33912-7" @default.
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