Matches in SemOpenAlex for { <https://semopenalex.org/work/W4306410010> ?p ?o ?g. }
- W4306410010 abstract "Abstract Hydration control of structure and mechanical properties is a process widely exploited in living organisms for key biological functions and, most recently, also in man‐made smart materials. Here, the challenge of unveiling the underlying atomistic mechanisms of this phenomenon using all‐atom Molecular Dynamics (MD) simulations to model the hygroscopic properties of polymer‐brushes composed by single‐stranded DNA (ssDNA) molecules is faced. The simulations identify three swelling regimes with a markedly different mechanical response. This evolution is produced by the competition between the formation of additional water–ssDNA and water–water hydrogen bonds, in a subtle interplay with the co‐evolving structure of the ssDNA SAM. This cooperative interaction between conformational and hydration degrees of freedom should be applicable to other polymer brushes and related hydrogen‐bonded systems. The results have direct implications for the use of ssDNA SAMs as sequencing devices, explaining the crucial role of the polymer‐brush density in the SAM collective response to hydration, and for the alternative design of hygroscopic materials, that exploit the extreme hygroscopic power of biological polymers like ssDNA brushes." @default.
- W4306410010 created "2022-10-17" @default.
- W4306410010 creator A5009130188 @default.
- W4306410010 creator A5029849662 @default.
- W4306410010 creator A5040965179 @default.
- W4306410010 date "2022-10-17" @default.
- W4306410010 modified "2023-10-15" @default.
- W4306410010 title "Hygroscopy of Single‐Stranded DNA Nano‐Brushes: Atomic Workings of its Hydration‐Induced Deformation" @default.
- W4306410010 cites W1539434723 @default.
- W4306410010 cites W1675132674 @default.
- W4306410010 cites W1972342797 @default.
- W4306410010 cites W1976499671 @default.
- W4306410010 cites W1977367857 @default.
- W4306410010 cites W1983133073 @default.
- W4306410010 cites W1994941561 @default.
- W4306410010 cites W1997622681 @default.
- W4306410010 cites W2004822259 @default.
- W4306410010 cites W2005457526 @default.
- W4306410010 cites W2014954784 @default.
- W4306410010 cites W2021540635 @default.
- W4306410010 cites W2023936383 @default.
- W4306410010 cites W2030552522 @default.
- W4306410010 cites W2035687084 @default.
- W4306410010 cites W2050595677 @default.
- W4306410010 cites W2056211855 @default.
- W4306410010 cites W2061885535 @default.
- W4306410010 cites W2063831812 @default.
- W4306410010 cites W2068466911 @default.
- W4306410010 cites W2072282741 @default.
- W4306410010 cites W2082909620 @default.
- W4306410010 cites W2088821590 @default.
- W4306410010 cites W2089178093 @default.
- W4306410010 cites W2099045194 @default.
- W4306410010 cites W2108187138 @default.
- W4306410010 cites W2117228527 @default.
- W4306410010 cites W2121631837 @default.
- W4306410010 cites W2124499032 @default.
- W4306410010 cites W2130681953 @default.
- W4306410010 cites W2136729627 @default.
- W4306410010 cites W2141812131 @default.
- W4306410010 cites W2147993766 @default.
- W4306410010 cites W2165330698 @default.
- W4306410010 cites W2169802997 @default.
- W4306410010 cites W2209946376 @default.
- W4306410010 cites W2296919452 @default.
- W4306410010 cites W2299659008 @default.
- W4306410010 cites W2313116527 @default.
- W4306410010 cites W2324491933 @default.
- W4306410010 cites W2330405198 @default.
- W4306410010 cites W2332712348 @default.
- W4306410010 cites W2346438291 @default.
- W4306410010 cites W2408988793 @default.
- W4306410010 cites W2469187505 @default.
- W4306410010 cites W2509655505 @default.
- W4306410010 cites W2509889353 @default.
- W4306410010 cites W2517359652 @default.
- W4306410010 cites W2563913041 @default.
- W4306410010 cites W2601890660 @default.
- W4306410010 cites W2684748936 @default.
- W4306410010 cites W2760518623 @default.
- W4306410010 cites W2767331898 @default.
- W4306410010 cites W2778393669 @default.
- W4306410010 cites W2803512741 @default.
- W4306410010 cites W2809744867 @default.
- W4306410010 cites W2909145634 @default.
- W4306410010 cites W2911573580 @default.
- W4306410010 cites W2920113645 @default.
- W4306410010 cites W2938303314 @default.
- W4306410010 cites W3062046797 @default.
- W4306410010 cites W3097232373 @default.
- W4306410010 cites W3098294205 @default.
- W4306410010 cites W3098485836 @default.
- W4306410010 cites W3133802163 @default.
- W4306410010 cites W3180107556 @default.
- W4306410010 cites W3212997810 @default.
- W4306410010 cites W3216870933 @default.
- W4306410010 cites W4200056044 @default.
- W4306410010 cites W4234831805 @default.
- W4306410010 cites W4252709243 @default.
- W4306410010 doi "https://doi.org/10.1002/admi.202201272" @default.
- W4306410010 hasPublicationYear "2022" @default.
- W4306410010 type Work @default.
- W4306410010 citedByCount "1" @default.
- W4306410010 countsByYear W43064100102023 @default.
- W4306410010 crossrefType "journal-article" @default.
- W4306410010 hasAuthorship W4306410010A5009130188 @default.
- W4306410010 hasAuthorship W4306410010A5029849662 @default.
- W4306410010 hasAuthorship W4306410010A5040965179 @default.
- W4306410010 hasBestOaLocation W43064100101 @default.
- W4306410010 hasConcept C112887158 @default.
- W4306410010 hasConcept C147597530 @default.
- W4306410010 hasConcept C159467904 @default.
- W4306410010 hasConcept C159985019 @default.
- W4306410010 hasConcept C171250308 @default.
- W4306410010 hasConcept C178790620 @default.
- W4306410010 hasConcept C185592680 @default.
- W4306410010 hasConcept C192562407 @default.
- W4306410010 hasConcept C204366326 @default.
- W4306410010 hasConcept C207921521 @default.
- W4306410010 hasConcept C2778540859 @default.