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- W4306827031 endingPage "106520" @default.
- W4306827031 startingPage "106520" @default.
- W4306827031 abstract "Ionic liquids, owning multiple combinations of cations and anions, provide unique tunability for conducting polymer, which can provide distinctive properties tailored to different applications of these conducting polymer/ionic liquid composites. Herein, five different ionic liquids were utilized to dope poly (3, 4-ethylenedioxythiophene), PEDOT, affording five different PEDOT/ionic liquid composites, which were evaluated for their electrochemical sensing performance towards environmental pollutant nitrite. Among them, ionic liquid N , N -diethyl- N -methyl- N -(2-methoxyethyl) ammonium bis(trifluoromethanesulfonyl)imide ([Deme][NTf 2 ]) was unique in tuning PEDOT’s charge properties. No π - π intermolecular interactions were formed between bulky ammonium and PEDOT’s planar thiophene ring, thus cation [Deme] and anion [NTf 2 ] tended to compete for doping into PEDOT matrix. The bulky cation N , N -diethyl- N -methyl- N -(2-methoxyethyl)ammonium would remain more on PEDOT outside, affording more positive charge. The accumulated more positive charge on [Deme][NTf 2 ]-doped PEDOT’s surface was beneficial to attract more adsorption of nitrite anion, contributing to its improved electrochemical sensing performance. [Deme][NTf 2 ]-doped PEDOT was characterized by various techniques and served as excellent electrode modifier to enable nitrite determination, achieving a broad linear range of 0.05 to 10 mM and a high sensitivity of 642.38 μ A mM −1 cm −2 . Ionic liquid [Deme][NTf 2 ] demonstrated its unique tuning capabilities to afford conducting polymer/ionic liquid composite, aiming for promising electrochemical sensing application." @default.
- W4306827031 created "2022-10-20" @default.
- W4306827031 creator A5041205100 @default.
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- W4306827031 date "2022-10-01" @default.
- W4306827031 modified "2023-09-29" @default.
- W4306827031 title "Unique Tunability to Conducting Polymer Enabled by Ionic Liquid Doping and its Application in Nitrite Sensing" @default.
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- W4306827031 doi "https://doi.org/10.1149/1945-7111/ac9b99" @default.
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