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- W4306918346 abstract "Zirconium nitrate pentahydrate (Zr(NO3)4·5H2O) and tetraethyl orthosilicate (TEOS) are used as the zirconium source and silicon source, respectively, and methyltriethoxysilane (MTES) as the hydrophobic modifier; the hydrophilic and hydrophobic ZrO2-SiO2 xerogels were prepared successfully. The xerogels were characterized using Fourier transform infrared spectra (FTIR), X-ray diffraction (XRD), scanning electron microscopy (SEM), and N2 adsorption-desorption measurement. The adsorption mechanism of hydrophobic ZrO2-SiO2 xerogels to RhB was described by the kinetic and adsorption isotherms. The results showed that the introduction of Si-CH3 groups can make the average pore size, BET surface area, and total pore volume of ZrO2-SiO2 xerogel increase. The hydrophobic ZrO2-SiO2 xerogel displays an adsorption capacity of 169.23 mg·g-1 for RhB dye at 25 °C and pH = 3. The adsorption process of hydrophobic ZrO2-SiO2 xerogel to RhB followed a pseudo-second-order kinetic model. Fitting results from the D-R model of adsorption indicate that the adsorption of RhB onto the hydrophobic ZrO2-SiO2 xerogels is mainly physical, accompanied by a spontaneous heat absorption process. The regeneration and recycling properties of hydrophobic xerogels were investigated, and their recoverability and reusability were demonstrated." @default.
- W4306918346 created "2022-10-21" @default.
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- W4306918346 date "2022-10-20" @default.
- W4306918346 modified "2023-09-25" @default.
- W4306918346 title "Hydrophobic Modification of ZrO2-SiO2 Xerogel and Its Adsorption Properties to Rhodamine B" @default.
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- W4306918346 doi "https://doi.org/10.3390/gels8100675" @default.
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