Matches in SemOpenAlex for { <https://semopenalex.org/work/W4307169334> ?p ?o ?g. }
- W4307169334 abstract "We present an analytical pulse design protocol for controlling the vibrational dynamics of polar diatomic molecules within a given electronic state. Altering the potential energy function via the position-dependent electric permanent dipole moment, the vibrational state population dynamics is directly controlled using appropriately shaped laser pulses in the midinfrared regime. The optimal pulse shapes---that are expected to drive the molecule along user-defined quantum pathways---are obtained by reverse engineering, that is, solving the Schrodinger equation of the nuclei inversely in a relevant subspace. The proposed control scheme is validated by accurately solving the full time-dependent Schrodinger equation of the ${mathrm{HeH}}^{+}$ molecular ion with two completely different methods: (1) propagating the complex population amplitudes of many field-free eigenstates or (2) propagating directly the nuclear wave packet on a grid. We find that besides smooth transitions, arbitrary Rabi oscillations as well as vibrational ladder climbing can be efficiently controlled with the present scheme. As a result, the molecule is successively excited beyond the potential barrier, leading to enhanced dissociation in the ground electronic state. Rotational effects and possible extensions of the presented control are also briefly discussed." @default.
- W4307169334 created "2022-10-29" @default.
- W4307169334 creator A5003535638 @default.
- W4307169334 creator A5029303170 @default.
- W4307169334 date "2022-10-21" @default.
- W4307169334 modified "2023-10-16" @default.
- W4307169334 title "Coherent control of the vibrational dynamics of aligned heteronuclear diatomic molecules" @default.
- W4307169334 cites W1964688467 @default.
- W4307169334 cites W1980523056 @default.
- W4307169334 cites W1982899472 @default.
- W4307169334 cites W1983741956 @default.
- W4307169334 cites W1992188389 @default.
- W4307169334 cites W1993893336 @default.
- W4307169334 cites W1995765699 @default.
- W4307169334 cites W1996690830 @default.
- W4307169334 cites W2000002551 @default.
- W4307169334 cites W2001163906 @default.
- W4307169334 cites W2009977941 @default.
- W4307169334 cites W2022941775 @default.
- W4307169334 cites W2023821122 @default.
- W4307169334 cites W2026113886 @default.
- W4307169334 cites W2029283290 @default.
- W4307169334 cites W2031498216 @default.
- W4307169334 cites W2033483591 @default.
- W4307169334 cites W2037797326 @default.
- W4307169334 cites W2044522416 @default.
- W4307169334 cites W2045720759 @default.
- W4307169334 cites W2047876523 @default.
- W4307169334 cites W2048956787 @default.
- W4307169334 cites W2049366771 @default.
- W4307169334 cites W2049682393 @default.
- W4307169334 cites W2049823683 @default.
- W4307169334 cites W2053571266 @default.
- W4307169334 cites W2055842660 @default.
- W4307169334 cites W2060854320 @default.
- W4307169334 cites W2064955794 @default.
- W4307169334 cites W2066347451 @default.
- W4307169334 cites W2076372479 @default.
- W4307169334 cites W2079336704 @default.
- W4307169334 cites W2081407315 @default.
- W4307169334 cites W2087398666 @default.
- W4307169334 cites W2089294967 @default.
- W4307169334 cites W2091416857 @default.
- W4307169334 cites W2094706659 @default.
- W4307169334 cites W2103923649 @default.
- W4307169334 cites W2125993136 @default.
- W4307169334 cites W2133252865 @default.
- W4307169334 cites W2199969208 @default.
- W4307169334 cites W2225171054 @default.
- W4307169334 cites W2270640873 @default.
- W4307169334 cites W2321638212 @default.
- W4307169334 cites W2324999674 @default.
- W4307169334 cites W2327928778 @default.
- W4307169334 cites W2328287800 @default.
- W4307169334 cites W2409392049 @default.
- W4307169334 cites W2570989441 @default.
- W4307169334 cites W2593487957 @default.
- W4307169334 cites W2597436864 @default.
- W4307169334 cites W2614287864 @default.
- W4307169334 cites W2773514732 @default.
- W4307169334 cites W2798719566 @default.
- W4307169334 cites W2803956701 @default.
- W4307169334 cites W2809445577 @default.
- W4307169334 cites W2810668972 @default.
- W4307169334 cites W2885566484 @default.
- W4307169334 cites W2888578743 @default.
- W4307169334 cites W2889137343 @default.
- W4307169334 cites W2901878788 @default.
- W4307169334 cites W2908269171 @default.
- W4307169334 cites W2914701796 @default.
- W4307169334 cites W2937049145 @default.
- W4307169334 cites W2946720091 @default.
- W4307169334 cites W2964083768 @default.
- W4307169334 cites W2969212551 @default.
- W4307169334 cites W2970465500 @default.
- W4307169334 cites W2987682793 @default.
- W4307169334 cites W3006439213 @default.
- W4307169334 cites W3009229181 @default.
- W4307169334 cites W3034544861 @default.
- W4307169334 cites W3035506956 @default.
- W4307169334 cites W3099336136 @default.
- W4307169334 cites W3100505554 @default.
- W4307169334 cites W3108904002 @default.
- W4307169334 cites W3114362178 @default.
- W4307169334 cites W3135030843 @default.
- W4307169334 cites W3183491225 @default.
- W4307169334 cites W3204811794 @default.
- W4307169334 cites W4200130200 @default.
- W4307169334 cites W4200595481 @default.
- W4307169334 cites W4205627518 @default.
- W4307169334 cites W4210721717 @default.
- W4307169334 cites W4212838443 @default.
- W4307169334 cites W4226326030 @default.
- W4307169334 cites W4282930448 @default.
- W4307169334 cites W4282979520 @default.
- W4307169334 cites W4312741474 @default.
- W4307169334 doi "https://doi.org/10.1103/physreva.106.043113" @default.
- W4307169334 hasPublicationYear "2022" @default.
- W4307169334 type Work @default.
- W4307169334 citedByCount "1" @default.