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- W4307227922 abstract "Photoresponsive batteries promise flexible and low-cost solar-to-electrochemical energy storage (SES), but suffer from a limited SES efficiency due to rapid charge recombination and sluggish redox. Here, we present a porous-shell/core hybrid of covalent organic framework@carbon nanotube. This hybrid ensures long-lived separated charges (τave =3.0 ns) by an electron transfer relay starting from the donor-acceptor molecules to the nanoscale heterojunction. These charges are further allowed to drive high-rate redox of -C=O/-C-O- and -C-N/-C=N+ with facile kinetics. Equipped with this photoelectrochemical cathode, a photoresponsive aqueous battery shows a 5-fold enhancement in SES efficiency (1.1 % at 1 sun) over their counterparts. It is unveiled that the electron relay favors the formation of electron-enriching -C-O- and hole-enriching -C=N+ groups responsible for photoelectrochemical Zn2+ and OTf- storage cascade; and further, the general photo coupled ions transfer (PCIT) process is proposed. This work presents an inspiring photoelectrochemical cathode design and theoretical insight for photoresponsive batteries." @default.
- W4307227922 created "2022-10-30" @default.
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- W4307227922 date "2022-11-17" @default.
- W4307227922 modified "2023-10-17" @default.
- W4307227922 title "A Photoresponsive Battery Based on a Redox‐Coupled Covalent‐Organic‐Framework Hybrid Photoelectrochemical Cathode" @default.
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- W4307227922 doi "https://doi.org/10.1002/anie.202214816" @default.
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