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- W4307282757 abstract "We construct an information-geometric structure for chemical thermodynamics, applicable to a wide range of chemical reaction systems including nonideal and open systems. For this purpose, we explicitly construct dual affine coordinate systems, which completely designate an information-geometric structure, using the extent of reactions and the affinities of reactions as coordinates on a linearly constrained space of amounts of substances. The resulting structure induces a metric and a divergence (a function of two distributions of amounts), both expressed with chemical potentials. These quantities have been partially known for ideal-dilute solutions, but their extensions for nonideal solutions and the complete underlying structure are novel. The constructed geometry is a generalization of dual affine coordinates for stochastic thermodynamics. For example, the metric and the divergence are generalizations of the Fisher information and the Kullback-Leibler divergence. As an application, we identify the chemical-thermodynamic analog of the Hatano-Sasa excess entropy production using our divergence." @default.
- W4307282757 created "2022-10-31" @default.
- W4307282757 creator A5001457441 @default.
- W4307282757 creator A5003434104 @default.
- W4307282757 date "2022-10-24" @default.
- W4307282757 modified "2023-10-14" @default.
- W4307282757 title "Information-geometric structure for chemical thermodynamics: An explicit construction of dual affine coordinates" @default.
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- W4307282757 doi "https://doi.org/10.1103/physreve.106.044131" @default.
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