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• W4307500036 abstract "Trivalent group-9 metal catalysts with a cyclopentadienyl-type ligand (CpMIII ; M=Co, Rh, Ir, Cp=cyclopentadienyl) have been widely used for directed C-H functionalizations, albeit that their application to challenging C(sp3 )-H functionalizations suffers from the limitations of the available directing groups. In this report, we describe directed C(sp3 )-H amidation reactions of simple amide substrates with a variety of substituents. The combination of an electron-deficient CpE Rh catalyst (CpE =1,3-bis(ethoxycarbonyl)-substituted Cp) and an electron-deficient 2-pyridone ligand is essential for high reactivity." @default.
• W4307500036 created "2022-11-02" @default.
• W4307500036 creator A5012058996 @default.
• W4307500036 creator A5013437976 @default.
• W4307500036 creator A5015482405 @default.
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• W4307500036 creator A5039511820 @default.
• W4307500036 creator A5048672449 @default.
• W4307500036 creator A5052530886 @default.
• W4307500036 creator A5074774949 @default.
• W4307500036 creator A5087150556 @default.
• W4307500036 date "2022-11-23" @default.
• W4307500036 modified "2023-10-16" @default.
• W4307500036 title "Native Amide‐Directed C(sp ³ )−H Amidation Enabled by Electron‐Deficient Rh ^III Catalyst and Electron‐Deficient 2‐Pyridone Ligand" @default.
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