FRINK Linked Data Fragments server

Matches in SemOpenAlex for { <https://semopenalex.org/work/W4307645002> ?p ?o ?g. }

• W4307645002 endingPage "1224" @default.
• W4307645002 startingPage "1217" @default.
• W4307645002 abstract "Lithium-metal batteries are a promising technology to address the emerging demand for high-energy-density storage systems. However, their cycling encounters a low Coulombic efficiency (CE) due to the unceasing electrolyte decomposition. Improving the stability of solid electrolyte interphase (SEI) suppresses the decomposition and increases CE. However, SEI morphology and chemistry alone cannot account for CE, and a full explanation is still lacking. Here we report that in diverse electrolytes, the large shift (>0.6 V) in the Li electrode potential and its association with the Li+ coordination structure influence the CE. Machine learning regression analysis and vibrational spectroscopy revealed that the formation of ion pairs is essential for upshifting the Li electrode potential, that is, for weakening the reducing ability of Li, which would lead to a high CE with diminished electrolyte decomposition. Various electrolytes with enhanced ion-pairing solution structure are designed to enable a significantly improved CE (>99%). It is a challenging task to understand the reversibility of lithium-metal anodes in batteries. Here the authors identify the lithium electrode potential as a critical factor that affects the anode reversibility and subsequently propose an electrolyte design to improve the cycling performance." @default.
• W4307645002 created "2022-11-04" @default.
• W4307645002 creator A5023575100 @default.
• W4307645002 creator A5041044598 @default.
• W4307645002 creator A5041748597 @default.
• W4307645002 creator A5057246100 @default.
• W4307645002 creator A5065511550 @default.
• W4307645002 creator A5069977540 @default.
• W4307645002 creator A5079334714 @default.
• W4307645002 date "2022-10-27" @default.
• W4307645002 modified "2023-10-16" @default.
• W4307645002 title "Electrode potential influences the reversibility of lithium-metal anodes" @default.
• W4307645002 cites W1594329901 @default.
• W4307645002 cites W1967244854 @default.
• W4307645002 cites W1970581450 @default.
• W4307645002 cites W1989632287 @default.
• W4307645002 cites W2007302339 @default.
• W4307645002 cites W2066387129 @default.
• W4307645002 cites W2071923033 @default.
• W4307645002 cites W2120145199 @default.
• W4307645002 cites W2121710229 @default.
• W4307645002 cites W2147993766 @default.
• W4307645002 cites W2155489103 @default.
• W4307645002 cites W2159744994 @default.
• W4307645002 cites W2172574721 @default.
• W4307645002 cites W2323318378 @default.
• W4307645002 cites W2328896751 @default.
• W4307645002 cites W2341894171 @default.
• W4307645002 cites W2342475091 @default.
• W4307645002 cites W2510164568 @default.
• W4307645002 cites W2514147873 @default.
• W4307645002 cites W2593815020 @default.
• W4307645002 cites W2744368717 @default.
• W4307645002 cites W2756200313 @default.
• W4307645002 cites W2774731903 @default.
• W4307645002 cites W2796223544 @default.
• W4307645002 cites W2810854392 @default.
• W4307645002 cites W2895630921 @default.
• W4307645002 cites W2930260497 @default.
• W4307645002 cites W2946737050 @default.
• W4307645002 cites W2953265075 @default.
• W4307645002 cites W2979220658 @default.
• W4307645002 cites W3015605954 @default.
• W4307645002 cites W3035811909 @default.
• W4307645002 cites W3174242950 @default.
• W4307645002 cites W3177210207 @default.
• W4307645002 cites W4205652915 @default.
• W4307645002 doi "https://doi.org/10.1038/s41560-022-01144-0" @default.
• W4307645002 hasPublicationYear "2022" @default.
• W4307645002 type Work @default.
• W4307645002 citedByCount "34" @default.
• W4307645002 countsByYear W43076450022022 @default.
• W4307645002 countsByYear W43076450022023 @default.
• W4307645002 crossrefType "journal-article" @default.
• W4307645002 hasAuthorship W4307645002A5023575100 @default.
• W4307645002 hasAuthorship W4307645002A5041044598 @default.
• W4307645002 hasAuthorship W4307645002A5041748597 @default.
• W4307645002 hasAuthorship W4307645002A5057246100 @default.
• W4307645002 hasAuthorship W4307645002A5065511550 @default.
• W4307645002 hasAuthorship W4307645002A5069977540 @default.
• W4307645002 hasAuthorship W4307645002A5079334714 @default.
• W4307645002 hasBestOaLocation W43076450022 @default.
• W4307645002 hasConcept C124681953 @default.
• W4307645002 hasConcept C127413603 @default.
• W4307645002 hasConcept C130349721 @default.
• W4307645002 hasConcept C134018914 @default.
• W4307645002 hasConcept C147789679 @default.
• W4307645002 hasConcept C17525397 @default.
• W4307645002 hasConcept C178790620 @default.
• W4307645002 hasConcept C179104552 @default.
• W4307645002 hasConcept C185592680 @default.
• W4307645002 hasConcept C192562407 @default.
• W4307645002 hasConcept C2778541603 @default.
• W4307645002 hasConcept C42360764 @default.
• W4307645002 hasConcept C68801617 @default.
• W4307645002 hasConcept C71924100 @default.
• W4307645002 hasConcept C89395315 @default.
• W4307645002 hasConceptScore W4307645002C124681953 @default.
• W4307645002 hasConceptScore W4307645002C127413603 @default.
• W4307645002 hasConceptScore W4307645002C130349721 @default.
• W4307645002 hasConceptScore W4307645002C134018914 @default.
• W4307645002 hasConceptScore W4307645002C147789679 @default.
• W4307645002 hasConceptScore W4307645002C17525397 @default.
• W4307645002 hasConceptScore W4307645002C178790620 @default.
• W4307645002 hasConceptScore W4307645002C179104552 @default.
• W4307645002 hasConceptScore W4307645002C185592680 @default.
• W4307645002 hasConceptScore W4307645002C192562407 @default.
• W4307645002 hasConceptScore W4307645002C2778541603 @default.
• W4307645002 hasConceptScore W4307645002C42360764 @default.
• W4307645002 hasConceptScore W4307645002C68801617 @default.
• W4307645002 hasConceptScore W4307645002C71924100 @default.
• W4307645002 hasConceptScore W4307645002C89395315 @default.
• W4307645002 hasIssue "12" @default.
• W4307645002 hasLocation W43076450021 @default.
• W4307645002 hasLocation W43076450022 @default.
• W4307645002 hasOpenAccess W4307645002 @default.
• W4307645002 hasPrimaryLocation W43076450021 @default.
• W4307645002 hasRelatedWork W2054530605 @default.

• next