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- W4307771059 abstract "Photoreactive coordination polymers are particularly important media for the implementation of highly-selective photoreactions and creation of photoresponsive intelligent materials and devices. Herein, a two-dimensional (2D) photoreactive coordination polymer, formulated as [Cd(pha)(3,3'-bpe)]n (1) was prepared through the hydrothermal reaction between Cd(NO3)2·4H2O, phthalic acid (H2pha) and 1,2-bis(3-pyridyl)ethylene (3,3'-bpe). Upon exposure to 365 nm UV light, the 1H NMR spectroscopy and single crystal X-ray diffraction analysis results indicated that 1 can undergo a [2 + 2] photocycloaddition reaction and thus form a new coordination polymer [Cd(pha)(3,3'-tpcb)0.5]n (1a) through single-crystal to single-crystal (SCSC) transformation. Accompanied by the SCSC photoreaction, the 2D sql net of 1 converted into a 2D binodal network of 1a with the rare (324·627)(326272) topology. The SCSC transformation from 1 to 1a also exhibits an interesting photocontrolled fluorescence. The unique photoinduced structural change and fluorescence quenching of 1 makes it a potential intelligent material for optical anti-counterfeiting, fluorescence sensors and other fields." @default.
- W4307771059 created "2022-11-05" @default.
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- W4307771059 date "2022-01-01" @default.
- W4307771059 modified "2023-10-04" @default.
- W4307771059 title "Topological structural transformation of a two-dimensional coordination polymer <i>via</i> single-crystal to single-crystal photoreaction" @default.
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- W4307771059 doi "https://doi.org/10.1039/d2dt03063b" @default.
- W4307771059 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36314637" @default.
- W4307771059 hasPublicationYear "2022" @default.
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