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• W4307771789 abstract "Water-soluble multinuclear complexes based on ruthenium 2,2'-bipyridine-6,6'-dicarboxylate (bda) and ditopic bipyridine linker units are investigated in three-component visible light-driven water oxidation catalysis. Systematic studies revealed a strong enhancement of the catalytic efficiency in the absence of organic co-solvents and with increasing oligomer length. In-depth kinetic and morphological investigations suggest that the enhanced performance is induced by the self-assembly of linear Ru(bda) oligomers into aggregated superstructures. The obtained turnover frequencies (up to 14.9 s-1 ) and turnover numbers (more than 1000) per ruthenium center are the highest reported so far for Ru(bda)-based photocatalytic water oxidation systems." @default.
• W4307771789 created "2022-11-05" @default.
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• W4307771789 date "2022-11-23" @default.
• W4307771789 modified "2023-09-30" @default.
• W4307771789 title "Self‐assembled Ru(bda) Coordination Oligomers as Efficient Catalysts for Visible Light‐Driven Water Oxidation in Pure Water" @default.
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• W4307771789 doi "https://doi.org/10.1002/anie.202211445" @default.
• W4307771789 hasPubMedId "https://pubmed.ncbi.nlm.nih.gov/36315034" @default.
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